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Cre activity converts cells from mtdTomato to mEGFP expression. ??b??, The timeline of the LNP-Cre delivery experiments. ??c?? ??e??\, Cre mRNA delivery to adult \(>5 	:196)/F 4/H/N/Rect[249.114 410.02 265.435 399.84]/Subtype/Link/Type/Annot>>endobj283 0 obj<</AP<</N 970 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??????????????Fig. 5???? |???? ??????LNP delivery testing in ferret model.???? ??????a??, Ferret Cre reporter mode\l. Cre activity converts cells from mtdTomato to mEGFP expression. ??b??, The timeline of the LNP-Cre delivery experiments. ??c?? ??e\??, Cre mRNA delivery to adult \(>5:197)/F 4/H/N/Rect[253.847 399.27 262.342 389.09]/Subtype/Link/Type/Annot>>endobj286 0 obj<</AP<</N 971 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:????38.????	??????????Yuan, F. et al. Transgenic ferret models define pulmonary ionocyte diversity and \function. ??Nature?? ??621??, 857 867 \(2023\).??\r:198)/F 4/H/N/Rect[202.148 388.52 207.71 378.34]/Subtype/Link/Type/Annot>>endobj289 0 obj<</AP<</N 972 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??56.????	??????????Fischer, A. J. et al. Mucus strands from submucosal glands initiate mucociliary tr\ansport of large particles. ??JCI Insight?? ??4??, e124863 \(2019\).??\r:199)/F 4/H/N/Rect[209.079 388.52 214.466 378.34]/Subtype/Link/Type/Annot>>endobj293 0 obj<</AP<</N 973 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??57.????	??????????Ostedgaard, L. S. et al. Lack of airway submucosal glands impairs respiratory host\ defenses. ??eLife?? ??9??, e59653 \(2020\).??\r:200)/F 4/H/N/Rect[215.834 388.52 220.586 378.34]/Subtype/Link/Type/Annot>>endobj297 0 obj<</AP<</N 974 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??????????????Fig. 4???? |???? ??????Respiratory tract delivery.???? ??????a??, IN FFL delivery \(1.5 	?g dose, ??n?? 	\= 	4\) comparison between lead DL candidates \(FO-32, FO-35 and EB-66\) and controls \(cKK-E12, SM-102 and lipid 331\). ??b??, OPA FF\L delivery comparison \(1 	?g dose, ??n:201)/F 4/H/N/Rect[117.355 367.02 125.2 356.84]/Subtype/Link/Type/Annot>>endobj301 0 obj<</AP<</N 975 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??58.????	??????????Tata, P. R. & Rajagopal, J. 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Model.?? ??64??, 9 17 \(2024\).??\r:151)/F 4/H/N/Rect[553.34 689.52 559.032 679.34]/Subtype/Link/Type/Annot>>endobj20 0 obj<</AP<</N 1096 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:????????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of avail\able LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a pr\edictive message-passing neural n:152)/F 4/H/N/Rect[425.674 657.27 434.089 647.09]/Subtype/Link/Type/Annot>>endobj24 0 obj<</AP<</N 1097 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??????????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of avai\lable LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a p\redictive message-passing neural :153)/F 4/H/N/Rect[466.276 603.52 473.239 593.34]/Subtype/Link/Type/Annot>>endobj28 0 obj<</AP<</N 1098 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??51.????	??????????Wu, Z. et al. MoleculeNet: a benchmark for molecular machine learning. ??Chem. Sci.?\? ??9??, 513 530 \(2018\).??\r:154)/F 4/H/N/Rect[380.513 549.77 385.177 539.59]/Subtype/Link/Type/Annot>>endobj32 0 obj<</AP<</N 1099 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:????????????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of ava\ilable LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a \predictive message-passing neural:155)/F 4/H/N/Rect[548.178 474.52 556.155 464.34]/Subtype/Link/Type/Annot>>endobj36 0 obj<</AP<</N 1100 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??????????35.????	??????????Rhym, L. H., Manan, R. S., Koller, A., Stephanie, G. & Anderson, D. G. Peptide\-encoding mRNA barcodes for the high-throughput in vivo screening of libraries of lipid nanoparticles for mRNA delivery. ??Nat. 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A deep learning approach to antibiotic discovery. ??Cell?? ??180?\?, 688 702.e13 \(2020\).??\r:115)/F 4/H/N/Rect[279.354 711.02 284.747 700.84]/Subtype/Link/Type/Annot>>endobj84 0 obj<</AP<</N 1112 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??32.????	??????????Reker, D. et al. Computationally guided high-throughput design of self-assembling \drug nanoparticles. ??Nat. Nanotechnol.?? ??16??, 725 733 \(2021\).??\r:116)/F 4/H/N/Rect[287.494 711.02 292.62 700.84]/Subtype/Link/Type/Annot>>endobj88 0 obj<</AP<</N 1113 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??30.????	??????????Yang, K. et al. Analyzing learned molecular representations for property predictio\n. ??J. Chem. Inf. Model.?? ??59??, 3370 3388 \(2019\).??\r:117)/F 4/H/N/Rect[146.72 678.77 152.648 668.59]/Subtype/Link/Type/Annot>>endobj92 0 obj<</AP<</N 1114 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:????29.????	??????????Stokes, J. M. et al. A deep learning approach to antibiotic discovery. ??Cell?? ??18\0??, 688 702.e13 \(2020\).??\r:118)/F 4/H/N/Rect[80.2129 668.02 85.2157 657.84]/Subtype/Link/Type/Annot>>endobj96 0 obj<</AP<</N 1115 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??33.????	??????????Liu, G. et al. Deep learning-guided discovery of an antibiotic targeting ??Acinetob\acter baumannii??. ??Nat. Chem. Biol.?? ??19??, 1342 1350 \(2023\).??\r:119)/F 4/H/N/Rect[86.574 668.02 91.7829 657.84]/Subtype/Link/Type/Annot>>endobj100 0 obj<</AP<</N 1116 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??34.????	??????????Wong, F. et al. Discovery of a structural class of antibiotics with explainable de\ep learning. ??Nature?? ??626??, 177 185 \(2024\).??\r:120)/F 4/H/N/Rect[93.1412 668.02 98.7604 657.84]/Subtype/Link/Type/Annot>>endobj104 0 obj<</AP<</N 1117 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:????28.????	??????????Li, B. et al. Accelerating ionizable lipid discovery for mRNA delivery using mach\ine learning and combinatorial chemistry. ??Nat. Mater.?? ??23??, 1002 1008 \(2024\).??\r:121)/F 4/H/N/Rect[249.788 646.52 255.386 636.34]/Subtype/Link/Type/Annot>>endobj108 0 obj<</AP<</N 1118 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??35.????	??????????Rhym, L. H., Manan, R. S., Koller, A., Stephanie, G. & Anderson, D. G. Peptide-enc\oding mRNA barcodes for the high-throughput in vivo screening of libraries of lipid nanoparticles for mRNA delivery. ??Nat. Biome\d. Eng.?? ??7??, 901 910 \(2023\).??\r:122)/F 4/H/N/Rect[135.289 592.77 140.358 582.59]/Subtype/Link/Type/Annot>>endobj112 0 obj<</AP<</N 1119 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??????1.????	??????????Hou, X., Zaks, T., Langer, R. & Dong, Y. Lipid nanoparticles for mRNA delivery. ??\Nat. Rev. Mater.?? ??6??, 1078 1094 \(2021\).??\r:123)/F 4/H/N/Rect[292.753 571.27 294.803 561.09]/Subtype/Link/Type/Annot>>endobj116 0 obj<</AP<</N 1120 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??????24.????	??????????Sabnis, S. et al. A novel amino lipid series for mRNA delivery: improved endosom\al escape and sustained pharmacology and safety in non-human primates. ??Mol. 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Med.?? ??380??, 1941 1953\ \(2019\).??\r:128)/F 4/H/N/Rect[212.469 388.52 218.523 378.34]/Subtype/Link/Type/Annot>>endobj136 0 obj<</AP<</N 1125 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of available \LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a predict\ive message-passing neural networ:129)/F 4/H/N/Rect[58.4869 302.52 66.3509 292.34]/Subtype/Link/Type/Annot>>endobj140 0 obj<</AP<</N 1126 0 R>>/BS<</S/S/Type/Border/W 0>>/Border[0 0 0]/Dest(??springernature_natbio_2490.indd:??????15.????	??????????Miao, L. et al. Delivery of mRNA vaccines with heterocyclic lipids increases ant\i-tumor efficacy by STING-mediated immune cell activation. ??Nat. 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endstreamendobj874 0 obj<</A 566 0 R/C[0.0 0.0 0.0]/Count 17/F 0/First 1199 0 R/Last 1200 0 R/Parent 872 0 R/Title(??Artificial intelligence-guided design of lipid nanoparticles for pulmonary gene therapy\r)>>endobj566 0 obj<</D(springernature_natbio_2490.indd:Anchor 1:53)/S/GoTo>>endobj1199 0 obj<</A 614 0 R/C[0.0 0.0 0.0]/Count 8/F 0/First 1201 0 R/Last 1202 0 R/Next 1203 0 R/Parent 874 0 R/Title(??Results\r)>>endobj1200 0 obj<</A 574 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Parent 874 0 R/Prev 1204 0 R/Title(??Table 1 The percentage of GFP+ cells out of the total number of bronchial epithelial cells in manually selected, highly transf\ected bronchi for each lobe, carina and trachea.)>>endobj574 0 obj<</D(springernature_natbio_2490.indd:Anchor 18:70)/S/GoTo>>endobj1204 0 obj<</A 579 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1200 0 R/Parent 874 0 R/Prev 1205 0 R/Title(??Fig. 5 LNP delivery testing in ferret model.)>>endobj579 0 obj<</D(springernature_natbio_2490.indd:Anchor 17:69)/S/GoTo>>endobj1205 0 obj<</A 584 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1204 0 R/Parent 874 0 R/Prev 1206 0 R/Title(??Fig. 4 Respiratory tract delivery.)>>endobj584 0 obj<</D(springernature_natbio_2490.indd:Anchor 16:68)/S/GoTo>>endobj1206 0 obj<</A 590 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1205 0 R/Parent 874 0 R/Prev 1207 0 R/Title(??Fig. 3 Combining LiON with 4CR chemistry.)>>endobj590 0 obj<</D(springernature_natbio_2490.indd:Anchor 15:67)/S/GoTo>>endobj1207 0 obj<</A 596 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1206 0 R/Parent 874 0 R/Prev 1208 0 R/Title(??Fig. 2 LiON for optimizing intravenous liver delivery of branched-ester-based library.)>>endobj596 0 obj<</D(springernature_natbio_2490.indd:Anchor 14:66)/S/GoTo>>endobj1208 0 obj<</A 602 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1207 0 R/Parent 874 0 R/Prev 1209 0 R/Title(??Fig. 1 Workflow for LiON, DL-based LNP design.)>>endobj602 0 obj<</D(springernature_natbio_2490.indd:Anchor 13:65)/S/GoTo>>endobj1209 0 obj<</A 608 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1208 0 R/Parent 874 0 R/Prev 1203 0 R/Title(??Online content\r)>>endobj608 0 obj<</D(springernature_natbio_2490.indd:Anchor 12:64)/S/GoTo>>endobj1203 0 obj<</A 612 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1209 0 R/Parent 874 0 R/Prev 1199 0 R/Title(??Discussion\r)>>endobj612 0 obj<</D(springernature_natbio_2490.indd:Anchor 11:63)/S/GoTo>>endobj614 0 obj<</D(springernature_natbio_2490.indd:Anchor 2:54)/S/GoTo>>endobj1201 0 obj<</A 660 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1210 0 R/Parent 1199 0 R/Title(??Dataset and DL model design\r)>>endobj1202 0 obj<</A 623 0 R/C[0.0 0.0 0.0]/Count 4/F 0/First 1211 0 R/Last 1212 0 R/Parent 1199 0 R/Prev 1213 0 R/Title(??Application of LiON to a novel four-component library\r)>>endobj623 0 obj<</D(springernature_natbio_2490.indd:Anchor 6:58)/S/GoTo>>endobj1211 0 obj<</A 657 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1214 0 R/Parent 1202 0 R/Title(??Design of lipids for intramuscular delivery)>>endobj1212 0 obj<</A 643 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Parent 1202 0 R/Prev 1215 0 R/Title(??LiON 2.0: streamlining and cross validation)>>endobj1213 0 obj<</A 634 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1202 0 R/Parent 1199 0 R/Prev 1210 0 R/Title(??Application of LiON to branched-ester library\r)>>endobj634 0 obj<</D(springernature_natbio_2490.indd:Anchor 5:57)/S/GoTo>>endobj1210 0 obj<</A 640 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1213 0 R/Parent 1199 0 R/Prev 1201 0 R/Title(??Design and characterization of the DL model for predicting LNP activity\r)>>endobj640 0 obj<</D(springernature_natbio_2490.indd:Anchor 4:56)/S/GoTo>>endobj643 0 obj<</D(springernature_natbio_2490.indd:Anchor 10:62)/S/GoTo>>endobj1215 0 obj<</A 648 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1212 0 R/Parent 1202 0 R/Prev 1214 0 R/Title(??Lipid structural analysis)>>endobj648 0 obj<</D(springernature_natbio_2490.indd:Anchor 9:61)/S/GoTo>>endobj1214 0 obj<</A 654 0 R/C[0.0 0.0 0.0]/Count 0/F 0/Next 1215 0 R/Parent 1202 0 R/Prev 1211 0 R/Title(??Lipid testing for respiratory tract delivery)>>endobj654 0 obj<</D(springernature_natbio_2490.indd:Anchor 8:60)/S/GoTo>>endobj657 0 obj<</D(springernature_natbio_2490.indd:Anchor 7:59)/S/GoTo>>endobj660 0 obj<</D(springernature_natbio_2490.indd:Anchor 3:55)/S/GoTo>>endobj696 0 obj<</Kids[699 0 R 702 0 R 705 0 R 708 0 R]>>endobj721 0 obj<<>>endobj699 0 obj<</Limits[(springernature_natbio_2490.indd:Anchor 10:62)(??springernature_natbio_2490.indd:??25.????	??????????Hashiba, K. et al. 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LNP ML. ??GitHub?? ????https://github.com/jswitten/LNP_ML???????? \\(2024\).??\r:239)[549 0 R/XYZ 305 638 null](??springernature_natbio_2490.indd:??????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of available \LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a predict\ive message-passing neural networ:129)[325 0 R/XYZ 39 269 null](??springernature_natbio_2490.indd:??????Fig. 2???? |???? ??????LiON for optimizing intravenous liver delivery of branched-ester-based libr\ary.???? ??????a??, Michael addition chemistry for generation of branched-tail ionizable lipids. DIC, ??N??,??N?? 2-di\(propan-2-yl\)methane\diimine; DMAP, 4-dimethylaminopyri:157)[565 0 R/XYZ 39 290 null](??springernature_natbio_2490.indd:??????Fig. 3???? |???? ??????Combining LiON with 4CR chemistry.???? ??????a??, A 4CR scheme to generate novel \ionizable lipids. ??b??, Initial intramuscular \(i.m.\) delivery testing with ML3 and ML5 \(1 	?g dose, BL/6 mice\) compared with cKK\-E12 \(??n?? 	= 	1 mouse per LNP injecte:169)[662 0 R/XYZ 39 214 null](??springernature_natbio_2490.indd:??????Fig. 4???? |???? ??????Respiratory tract delivery.???? ??????a??, IN FFL delivery \(1.5 	?g dose, ??n?? 	= 	4\)\ comparison between lead DL candidates \(FO-32, FO-35 and EB-66\) and controls \(cKK-E12, SM-102 and lipid 331\). ??b??, OPA FFL de\livery comparison \(1 	?g dose, ??n?? 	= 	:185)[689 0 R/XYZ 39 386 null](??springernature_natbio_2490.indd:??????Fig. 5???? |???? ??????LNP delivery testing in ferret model.???? ??????a??, Ferret Cre reporter model. C\re activity converts cells from mtdTomato to mEGFP expression. ??b??, The timeline of the LNP-Cre delivery experiments. ??c?? ??e??, C\re mRNA delivery to adult \(>5 	mon:193)[767 0 R/XYZ 39 309 null](??springernature_natbio_2490.indd:??????Table 1???? |???? ??????The percentage of GFP??+?? cells out of the total number of bronchial epithe\lial cells in manually selected, highly transfected bronchi for each lobe, carina and trachea??????\r????????????????????:204)[256 0 R/XYZ 39 746 null]]>>endobj708 0 obj<</Limits[(??springernature_natbio_2490.indd:????????1.????	??????????Hou, X., Zaks, T., Langer, R. & Dong, Y. Lipid nanoparticles for mRNA delivery. ?\?Nat. Rev. Mater.?? ??6??, 1078 1094 \(2021\).??\r:162)(??springernature_natbio_2490.indd:????????????????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of a\vailable LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, \a predictive message-passing neur:237)]/Names[(??springernature_natbio_2490.indd:????????1.????	??????????Hou, X., Zaks, T., Langer, R. & Dong, Y. Lipid nanoparticles for mRNA delivery. ?\?Nat. Rev. Mater.?? ??6??, 1078 1094 \(2021\).??\r:162)[478 0 R/XYZ 39 509 null](??springernature_natbio_2490.indd:????????14.????	??????????Choi, S. H. & Engelhardt, J. F. Gene therapy for cystic fibrosis: lessons learn\ed and paths forward. ??Mol. Ther.?? ??29??, 428 430 \n\(2021\).??\r:217)[478 0 R/XYZ 39 154 null](??springernature_natbio_2490.indd:????????15.????	??????????Miao, L. et al. Delivery of mRNA vaccines with heterocyclic lipids increases an\ti-tumor efficacy by STING-mediated immune cell activation. ??Nat. Biotechnol.?? ??37??, 1174 1185 \(2019\).??\r:144)[478 0 R/XYZ 39 122 null](??springernature_natbio_2490.indd:????????24.????	??????????Sabnis, S. et al. A novel amino lipid series for mRNA delivery: improved endoso\mal escape and sustained pharmacology and safety in non-human primates. ??Mol. Ther.?? ??26??, 1509 1519 \(2018\).??\r:164)[478 0 R/XYZ 305 487 null](??springernature_natbio_2490.indd:????????27.????	??????????Whitehead, K. A. et al. Degradable lipid nanoparticles with predictable in vivo\ siRNA delivery activity. ??Nat. Commun.?? ??5??, 4277 \(2014\).??\r:210)[478 0 R/XYZ 305 391 null](??springernature_natbio_2490.indd:????????35.????	??????????Rhym, L. H., Manan, R. S., Koller, A., Stephanie, G. & Anderson, D. G. Peptide-\encoding mRNA barcodes for the high-throughput in vivo screening of libraries of lipid nanoparticles for mRNA delivery. ??Nat. Bi\omed. Eng.?? ??7??, 901 910 \(2023\).??:150)[478 0 R/XYZ 305 165 null](??springernature_natbio_2490.indd:????????41.????	????Li, B. et al. Enhancing the immunogenicity of lipid-nanoparticle mRNA vaccines by \adjuvanting the ionizable lipid and the mRNA. ??Nat. Biomed. Eng??. ????https://doi.org/10.1038/s41551-023-01082-6???????? \(2023\).??\r:1\83)[549 0 R/XYZ 39 692 null](??springernature_natbio_2490.indd:????????42.????	??????????Jiang, A. Y. et al. Combinatorial development of nebulized mRNA delivery formul\ations for the lungs. ??Nat. Nanotechnol.?? ??19??, 364 375 \(2024\).??\r:191)[549 0 R/XYZ 39 649 null](??springernature_natbio_2490.indd:????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of available\ LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a predic\tive message-passing neural netwo:134)[325 0 R/XYZ 39 269 null](??springernature_natbio_2490.indd:????????Fig. 2???? |???? ??????LiON for optimizing intravenous liver delivery of branched-ester-based lib\rary.???? ??????a??, Michael addition chemistry for generation of branched-tail ionizable lipids. DIC, ??N??,??N?? 2-di\(propan-2-yl\)methan\ediimine; DMAP, 4-dimethylaminopyr:159)[565 0 R/XYZ 39 290 null](??springernature_natbio_2490.indd:????????Fig. 3???? |???? ??????Combining LiON with 4CR chemistry.???? ??????a??, A 4CR scheme to generate novel\ ionizable lipids. ??b??, Initial intramuscular \(i.m.\) delivery testing with ML3 and ML5 \(1 	?g dose, BL/6 mice\) compared with cK\K-E12 \(??n?? 	= 	1 mouse per LNP inject:174)[662 0 R/XYZ 39 214 null](??springernature_natbio_2490.indd:????????Fig. 4???? |???? ??????Respiratory tract delivery.???? ??????a??, IN FFL delivery \(1.5 	?g dose, ??n?? 	= 	4\\) comparison between lead DL candidates \(FO-32, FO-35 and EB-66\) and controls \(cKK-E12, SM-102 and lipid 331\). ??b??, OPA FFL d\elivery comparison \(1 	?g dose, ??n?? 	=:189)[689 0 R/XYZ 39 386 null](??springernature_natbio_2490.indd:????????Fig. 5???? |???? ??????LNP delivery testing in ferret model.???? ??????a??, Ferret Cre reporter model. \Cre activity converts cells from mtdTomato to mEGFP expression. ??b??, The timeline of the LNP-Cre delivery experiments. ??c?? ??e??, \Cre mRNA delivery to adult \(>5 	mo:194)[767 0 R/XYZ 39 309 null](??springernature_natbio_2490.indd:??????????1.????	??????????Hou, X., Zaks, T., Langer, R. & Dong, Y. Lipid nanoparticles for mRNA delivery.\ ??Nat. Rev. Mater.?? ??6??, 1078 1094 \(2021\).??\r:163)[478 0 R/XYZ 39 509 null](??springernature_natbio_2490.indd:??????????15.????	??????????Miao, L. et al. Delivery of mRNA vaccines with heterocyclic lipids increases a\nti-tumor efficacy by STING-mediated immune cell activation. ??Nat. Biotechnol.?? ??37??, 1174 1185 \(2019\).??\r:149)[478 0 R/XYZ 39 122 null](??springernature_natbio_2490.indd:??????????35.????	??????????Rhym, L. H., Manan, R. S., Koller, A., Stephanie, G. & Anderson, D. G. Peptide\-encoding mRNA barcodes for the high-throughput in vivo screening of libraries of lipid nanoparticles for mRNA delivery. ??Nat. B\iomed. Eng.?? ??7??, 901 910 \(2023\).:156)[478 0 R/XYZ 305 165 null](??springernature_natbio_2490.indd:??????????41.????	????Li, B. et al. Enhancing the immunogenicity of lipid-nanoparticle mRNA vaccines by\ adjuvanting the ionizable lipid and the mRNA. ??Nat. Biomed. Eng??. ????https://doi.org/10.1038/s41551-023-01082-6???????? \(2023\).??\r:\184)[549 0 R/XYZ 39 692 null](??springernature_natbio_2490.indd:??????????42.????	??????????Jiang, A. Y. et al. Combinatorial development of nebulized mRNA delivery formu\lations for the lungs. ??Nat. Nanotechnol.?? ??19??, 364 375 \(2024\).??\r:220)[549 0 R/XYZ 39 649 null](??springernature_natbio_2490.indd:??????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of availabl\e LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a predi\ctive message-passing neural netw:135)[325 0 R/XYZ 39 269 null](??springernature_natbio_2490.indd:??????????Fig. 2???? |???? ??????LiON for optimizing intravenous liver delivery of branched-ester-based li\brary.???? ??????a??, Michael addition chemistry for generation of branched-tail ionizable lipids. DIC, ??N??,??N?? 2-di\(propan-2-yl\)metha\nediimine; DMAP, 4-dimethylaminopy:160)[565 0 R/XYZ 39 290 null](??springernature_natbio_2490.indd:??????????Fig. 3???? |???? ??????Combining LiON with 4CR chemistry.???? ??????a??, A 4CR scheme to generate nove\l ionizable lipids. ??b??, Initial intramuscular \(i.m.\) delivery testing with ML3 and ML5 \(1 	?g dose, BL/6 mice\) compared with c\KK-E12 \(??n?? 	= 	1 mouse per LNP injec:175)[662 0 R/XYZ 39 214 null](??springernature_natbio_2490.indd:??????????Fig. 4???? |???? ??????Respiratory tract delivery.???? ??????a??, IN FFL delivery \(1.5 	?g dose, ??n?? 	= 	\4\) comparison between lead DL candidates \(FO-32, FO-35 and EB-66\) and controls \(cKK-E12, SM-102 and lipid 331\). ??b??, OPA FFL \delivery comparison \(1 	?g dose, ??n?? 	:190)[689 0 R/XYZ 39 386 null](??springernature_natbio_2490.indd:??????????Fig. 5???? |???? ??????LNP delivery testing in ferret model.???? ??????a??, Ferret Cre reporter model.\ Cre activity converts cells from mtdTomato to mEGFP expression. ??b??, The timeline of the LNP-Cre delivery experiments. ??c?? ??e??,\ Cre mRNA delivery to adult \(>5 	m:195)[767 0 R/XYZ 39 309 null](??springernature_natbio_2490.indd:????????????1.????	??????????Hou, X., Zaks, T., Langer, R. & Dong, Y. Lipid nanoparticles for mRNA delivery\. ??Nat. Rev. Mater.?? ??6??, 1078 1094 \(2021\).??\r:212)[478 0 R/XYZ 39 509 null](??springernature_natbio_2490.indd:????????????15.????	??????????Miao, L. et al. Delivery of mRNA vaccines with heterocyclic lipids increases \anti-tumor efficacy by STING-mediated immune cell activation. ??Nat. Biotechnol.?? ??37??, 1174 1185 \(2019\).??\r:170)[478 0 R/XYZ 39 122 null](??springernature_natbio_2490.indd:????????????35.????	??????????Rhym, L. H., Manan, R. S., Koller, A., Stephanie, G. & Anderson, D. G. Peptid\e-encoding mRNA barcodes for the high-throughput in vivo screening of libraries of lipid nanoparticles for mRNA delivery. ??Nat. \Biomed. Eng.?? ??7??, 901 910 \(2023\):168)[478 0 R/XYZ 305 165 null](??springernature_natbio_2490.indd:????????????41.????	????Li, B. et al. Enhancing the immunogenicity of lipid-nanoparticle mRNA vaccines b\y adjuvanting the ionizable lipid and the mRNA. ??Nat. Biomed. Eng??. ????https://doi.org/10.1038/s41551-023-01082-6???????? \(2023\).??\r\:207)[549 0 R/XYZ 39 692 null](??springernature_natbio_2490.indd:????????????42.????	??????????Jiang, A. Y. et al. Combinatorial development of nebulized mRNA delivery form\ulations for the lungs. ??Nat. Nanotechnol.?? ??19??, 364 375 \(2024\).??\r:230)[549 0 R/XYZ 39 649 null](??springernature_natbio_2490.indd:????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of availab\le LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a pred\ictive message-passing neural net:136)[325 0 R/XYZ 39 269 null](??springernature_natbio_2490.indd:????????????Fig. 2???? |???? ??????LiON for optimizing intravenous liver delivery of branched-ester-based l\ibrary.???? ??????a??, Michael addition chemistry for generation of branched-tail ionizable lipids. DIC, ??N??,??N?? 2-di\(propan-2-yl\)meth\anediimine; DMAP, 4-dimethylaminop:161)[565 0 R/XYZ 39 290 null](??springernature_natbio_2490.indd:????????????Fig. 3???? |???? ??????Combining LiON with 4CR chemistry.???? ??????a??, A 4CR scheme to generate nov\el ionizable lipids. ??b??, Initial intramuscular \(i.m.\) delivery testing with ML3 and ML5 \(1 	?g dose, BL/6 mice\) compared with \cKK-E12 \(??n?? 	= 	1 mouse per LNP inje:176)[662 0 R/XYZ 39 214 null](??springernature_natbio_2490.indd:????????????Fig. 4???? |???? ??????Respiratory tract delivery.???? ??????a??, IN FFL delivery \(1.5 	?g dose, ??n?? 	=\ 	4\) comparison between lead DL candidates \(FO-32, FO-35 and EB-66\) and controls \(cKK-E12, SM-102 and lipid 331\). ??b??, OPA FFL\ delivery comparison \(1 	?g dose, ??n??:192)[689 0 R/XYZ 39 386 null](??springernature_natbio_2490.indd:????????????Fig. 5???? |???? ??????LNP delivery testing in ferret model.???? ??????a??, Ferret Cre reporter model\. Cre activity converts cells from mtdTomato to mEGFP expression. ??b??, The timeline of the LNP-Cre delivery experiments. ??c?? ??e??\, Cre mRNA delivery to adult \(>5 	:196)[767 0 R/XYZ 39 309 null](??springernature_natbio_2490.indd:??????????????35.????	??????????Rhym, L. H., Manan, R. S., Koller, A., Stephanie, G. & Anderson, D. G. Pepti\de-encoding mRNA barcodes for the high-throughput in vivo screening of libraries of lipid nanoparticles for mRNA delivery. ??Nat.\ Biomed. Eng.?? ??7??, 901 910 \(2023:224)[478 0 R/XYZ 305 165 null](??springernature_natbio_2490.indd:??????????????41.????	????Li, B. et al. Enhancing the immunogenicity of lipid-nanoparticle mRNA vaccines \by adjuvanting the ionizable lipid and the mRNA. ??Nat. Biomed. Eng??. ????https://doi.org/10.1038/s41551-023-01082-6???????? \(2023\).??\r\:223)[549 0 R/XYZ 39 692 null](??springernature_natbio_2490.indd:??????????????42.????	??????????Jiang, A. Y. et al. Combinatorial development of nebulized mRNA delivery for\mulations for the lungs. ??Nat. Nanotechnol.?? ??19??, 364 375 \(2024\).??\r:231)[549 0 R/XYZ 39 649 null](??springernature_natbio_2490.indd:??????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of availa\ble LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a pre\dictive message-passing neural ne:137)[325 0 R/XYZ 39 269 null](??springernature_natbio_2490.indd:??????????????Fig. 2???? |???? ??????LiON for optimizing intravenous liver delivery of branched-ester-based \library.???? ??????a??, Michael addition chemistry for generation of branched-tail ionizable lipids. DIC, ??N??,??N?? 2-di\(propan-2-yl\)met\hanediimine; DMAP, 4-dimethylamino:165)[565 0 R/XYZ 39 290 null](??springernature_natbio_2490.indd:??????????????Fig. 3???? |???? ??????Combining LiON with 4CR chemistry.???? ??????a??, A 4CR scheme to generate no\vel ionizable lipids. ??b??, Initial intramuscular \(i.m.\) delivery testing with ML3 and ML5 \(1 	?g dose, BL/6 mice\) compared with\ cKK-E12 \(??n?? 	= 	1 mouse per LNP inj:177)[662 0 R/XYZ 39 214 null](??springernature_natbio_2490.indd:??????????????Fig. 4???? |???? ??????Respiratory tract delivery.???? ??????a??, IN FFL delivery \(1.5 	?g dose, ??n?? 	\= 	4\) comparison between lead DL candidates \(FO-32, FO-35 and EB-66\) and controls \(cKK-E12, SM-102 and lipid 331\). ??b??, OPA FF\L delivery comparison \(1 	?g dose, ??n:201)[689 0 R/XYZ 39 386 null](??springernature_natbio_2490.indd:??????????????Fig. 5???? |???? ??????LNP delivery testing in ferret model.???? ??????a??, Ferret Cre reporter mode\l. Cre activity converts cells from mtdTomato to mEGFP expression. ??b??, The timeline of the LNP-Cre delivery experiments. ??c?? ??e\??, Cre mRNA delivery to adult \(>5:197)[767 0 R/XYZ 39 309 null](??springernature_natbio_2490.indd:????????????????35.????	??????????Rhym, L. H., Manan, R. S., Koller, A., Stephanie, G. & Anderson, D. G. Pept\ide-encoding mRNA barcodes for the high-throughput in vivo screening of libraries of lipid nanoparticles for mRNA delivery. ??Nat\. Biomed. Eng.?? ??7??, 901 910 \(202:229)[478 0 R/XYZ 305 165 null](??springernature_natbio_2490.indd:????????????????42.????	??????????Jiang, A. Y. et al. Combinatorial development of nebulized mRNA delivery fo\rmulations for the lungs. ??Nat. Nanotechnol.?? ??19??, 364 375 \(2024\).??\r:233)[549 0 R/XYZ 39 649 null](??springernature_natbio_2490.indd:????????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of avail\able LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a pr\edictive message-passing neural n:152)[325 0 R/XYZ 39 269 null](??springernature_natbio_2490.indd:????????????????Fig. 2???? |???? ??????LiON for optimizing intravenous liver delivery of branched-ester-based\ library.???? ??????a??, Michael addition chemistry for generation of branched-tail ionizable lipids. DIC, ??N??,??N?? 2-di\(propan-2-yl\)me\thanediimine; DMAP, 4-dimethylamin:166)[565 0 R/XYZ 39 290 null](??springernature_natbio_2490.indd:????????????????Fig. 3???? |???? ??????Combining LiON with 4CR chemistry.???? ??????a??, A 4CR scheme to generate n\ovel ionizable lipids. ??b??, Initial intramuscular \(i.m.\) delivery testing with ML3 and ML5 \(1 	?g dose, BL/6 mice\) compared wit\h cKK-E12 \(??n?? 	= 	1 mouse per LNP in:178)[662 0 R/XYZ 39 214 null](??springernature_natbio_2490.indd:??????????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of avai\lable LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a p\redictive message-passing neural :153)[325 0 R/XYZ 39 269 null](??springernature_natbio_2490.indd:??????????????????Fig. 2???? |???? ??????LiON for optimizing intravenous liver delivery of branched-ester-base\d library.???? ??????a??, Michael addition chemistry for generation of branched-tail ionizable lipids. DIC, ??N??,??N?? 2-di\(propan-2-yl\)m\ethanediimine; DMAP, 4-dimethylami:167)[565 0 R/XYZ 39 290 null](??springernature_natbio_2490.indd:??????????????????Fig. 3???? |???? ??????Combining LiON with 4CR chemistry.???? ??????a??, A 4CR scheme to generate \novel ionizable lipids. ??b??, Initial intramuscular \(i.m.\) delivery testing with ML3 and ML5 \(1 	?g dose, BL/6 mice\) compared wi\th cKK-E12 \(??n?? 	= 	1 mouse per LNP i:179)[662 0 R/XYZ 39 214 null](??springernature_natbio_2490.indd:????????????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of ava\ilable LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a \predictive message-passing neural:155)[325 0 R/XYZ 39 269 null](??springernature_natbio_2490.indd:????????????????????Fig. 3???? |???? ??????Combining LiON with 4CR chemistry.???? ??????a??, A 4CR scheme to generate\ novel ionizable lipids. ??b??, Initial intramuscular \(i.m.\) delivery testing with ML3 and ML5 \(1 	?g dose, BL/6 mice\) compared w\ith cKK-E12 \(??n?? 	= 	1 mouse per LNP :226)[662 0 R/XYZ 39 214 null](??springernature_natbio_2490.indd:??????????????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of av\ailable LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, a\ predictive message-passing neura:158)[325 0 R/XYZ 39 269 null](??springernature_natbio_2490.indd:????????????????????????Fig. 1???? |???? ??????Workflow for LiON, DL-based LNP design.???? ??????a??, A collection of a\vailable LNP data, typically collected from a screen generated via combinatorial synthesis. ??b??, Schematic of training of LiON, \a predictive message-passing neur:237)[325 0 R/XYZ 39 269 null]]>>endobj663 0 obj<</BaseFont/Helvetica/Encoding 669 0 R/Name/Helv/Subtype/Type1/Type/Font>>endobj666 0 obj<</BaseFont/ZapfDingbats/Name/ZaDb/Subtype/Type1/Type/Font>>endobj669 0 obj<</Differences[24/breve/caron/circumflex/dotaccent/hungarumlaut/ogonek/ring/tilde 39/quotesingle 96/grave 128/bullet/dagger/daggerdbl/ellipsis/emdash/endash/florin/fraction/guilsinglleft/guilsinglright/minus/perthousand/quotedblbase/quotedblleft/quotedblright/quoteleft/quoteright/quotesinglbase/trademark/fi/fl/Lslash/OE/Scaron/Ydieresis/Zcaron/dotlessi/lslash/oe/scaron/zcaron 160/Euro 164/currency 166/brokenbar 168/dieresis/copyright/ordfeminine 172/logicalnot/.notdef/registered/macron/degree/plusminus/twosuperior/threesuperior/acute/mu 183/periodcentered/cedilla/onesuperior/ordmasculine 188/onequarter/onehalf/threequarters 192/Agrave/Aacute/Acircumflex/Atilde/Adieresis/Aring/AE/Ccedilla/Egrave/Eacute/Ecircumflex/Edieresis/Igrave/Iacute/Icircumflex/Idieresis/Eth/Ntilde/Ograve/Oacute/Ocircumflex/Otilde/Odieresis/multiply/Oslash/Ugrave/Uacute/Ucircumflex/Udieresis/Yacute/Thorn/germandbls/agrave/aacute/acircumflex/atilde/adieresis/aring/ae/ccedilla/egrave/eacute/ecircumflex/edieresis/igrave/iacute/icircumflex/idieresis/eth/ntilde/ograve/oacute/ocircumflex/otilde/odieresis/divide/oslash/ugrave/uacute/ucircumflex/udieresis/yacute/thorn/ydieresis]/Type/Encoding>>endobj1216 0 obj<</Author(Jacob Witten)/CreationDate(D:20241202211910+05'30')/Creator(Springer)/CrossMarkDomains#5B1#5D(springer.com)/CrossMarkDomains#5B2#5D(springerlink.com)/Keywords()/ModDate(D:20241202212026+05'30')/Subject(Nature Biotechnology, doi:10.1038/s41587-024-02490-y)/Title(Artificial intelligence-guided design of lipid nanoparticles for pulmonary gene therapy)/doi(10.1038/s41587-024-02490-y)>>endobjxref
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